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Abstract. Aerosol interactions with clouds represent a significant uncertainty in our understanding of the Earth system. Deep convective clouds may respond to aerosol perturbations in several ways that have proven difficult to elucidate with observations. Here, we leverage the two busiest maritime shipping lanes in the world, which emit aerosol particles and their precursors into an otherwise relatively clean tropical marine boundary layer, to make headway on the influence of aerosol on deep convective clouds. The recent 7-fold change in allowable fuel sulfur by the International Maritime Organization allows us to test the sensitivity of the lightning to changes in ship plume aerosol number-size distributions. We find that, across a range of atmospheric thermodynamic conditions, the previously documented enhancement of lightning over the shipping lanes has fallen by over 40 %. The enhancement is therefore at least partially aerosol-mediated, a conclusion that is supported by observations of droplet number at cloud base, which show a similar decline over the shipping lane. These results have fundamental implications for our understanding of aerosol–cloud interactions, suggesting that deep convective clouds are impacted by the aerosol number distribution in the remote marine environment. 

Abstract Aerosols are important environmental factors that can influence deep convective clouds (DCCs) by serving as cloud condensation nuclei. Due to complications in DCC dynamics and microphysics, and aerosol size distribution and composition, understanding aerosol‐DCC interactions has been a daunting challenge. Recently, the convective invigoration mechanisms through enhancing latent heating in condensation and ice‐related processes that have been proposed in literature are debated for their significance qualitatively and quantitatively. A salient issue arising from these debates is the imperative need to clarify essential knowledge and methodologies in investigating aerosol impacts on deep convection. Here we have presented our view of key aspects on investigating and understanding these invigoration mechanisms as well as the aerosol and meteorological conditions under which these mechanisms may be significant based on new findings. For example, the condensational invigoration is most significant under a clean condition with an introduction of a large number of ultrafine particles, and the freezing‐induced invigoration can be significant in a clean condition with a large number of relatively large‐size particles being added. We have made practical recommendations on approaches for investigating aerosol impacts on convection with both modeling and observations. We note that the feedback induced by the invigoration via the enhanced latent heating to circulation and meteorology can be an important part of aerosol impacts but is very complicated and varies with different convective storm types. This is an important future direction for studying aerosol‐DCC interactions. 

Abstract Exceptionally high‐energy lightning strokes >10⁶ J (X1000 stronger than average) in the very low‐frequency band between 5 and 18 kHz, also known as superbolts (SB), occur mostly during winter over the North‐East Atlantic, the Mediterranean Sea, and over the Altiplano in South America. Here we compare the World‐Wide Lightning Location Network database with meteorological and aerosol data to examine the causes of lightning stroke high energies. Our results show that the energy per stroke increases sharply as the distance between the cloud'scharging zone(where the cloud electrification occurs) and the surface decreases. Since thecharging zoneoccurs above the 0°C isotherm, this distance is shorter when the 0°C isotherm is closer to the surface. This occurs either due to cold air mass over the ocean during winter or high surface altitude in the Altiplano during summer thunderstorms. Stroke energy decreases with the warm phase of the cloud, as proxied by the cloud base temperature, and increases with a more developed cloud, as proxied by the cloud top temperature, but to a much lesser extent than the distance between the surface and 0°C isotherm. Aerosols play no significant role. It is hypothesized that a shorter distance between thecharging zoneand the ground represents less electrical resistance that allows stronger discharge currents. 

Abstract The known effects of thermodynamics and aerosols can well explain the thunderstorm activity over land, but fail over oceans. Here, tracking the full lifecycle of tropical deep convective cloud clusters shows that adding fine aerosols significantly increases the lightning density for a given rainfall amount over both ocean and land. In contrast, adding coarse sea salt (dry radius > 1 μm), known as sea spray, weakens the cloud vigor and lightning by producing fewer but larger cloud drops, which accelerate warm rain at the expense of mixed-phase precipitation. Adding coarse sea spray can reduce the lightning by 90% regardless of fine aerosol loading. These findings reconcile long outstanding questions about the differences between continental and marine thunderstorms, and help to understand lightning and underlying aerosol-cloud-precipitation interaction mechanisms and their climatic effects. 

Abstract. Aerosol–cloud interactions remain largely uncertain with respect to predicting theirimpacts on weather and climate. Cloud microphysics parameterization is oneof the factors leading to large uncertainty. Here, we investigate the impactsof anthropogenic aerosols on the convective intensity and precipitation of athunderstorm occurring on 19 June 2013 over Houston with the Chemistryversion of Weather Research and Forecast model (WRF-Chem) using the Morrisontwo-moment bulk scheme and spectral bin microphysics (SBM) scheme. We findthat the SBM predicts a deep convective cloud that shows better agreement withobservations in terms of reflectivity and precipitation compared with theMorrison bulk scheme that has been used in many weather and climate models.With the SBM scheme, we see a significant invigoration effect on convectiveintensity and precipitation by anthropogenic aerosols, mainly throughenhanced condensation latent heating. Such an effect is absent withthe Morrison two-moment bulk microphysics, mainly because the saturationadjustment approach for droplet condensation and evaporation calculationlimits the enhancement by aerosols in (1) condensation latent heat byremoving the dependence of condensation on droplets and aerosols and (2) ice-related processes because the approach leads to stronger warm rain andweaker ice processes than the explicit supersaturation approach. 

Abstract. Changes in land cover and aerosols resulting from urbanization may impactconvective clouds and precipitation. Here we investigate how Houstonurbanization can modify sea-breeze-induced convective cloud and precipitation through the urban land effect and anthropogenic aerosol effect. The simulations are carried out with the Chemistry version of the WeatherResearch and Forecasting model (WRF-Chem), which is coupled with spectral-bin microphysics (SBM) and the multilayer urban model with abuilding energy model (BEM-BEP). We find that Houston urbanization (thejoint effect of both urban land and anthropogenic aerosols) notably enhancesstorm intensity (by ∼ 75 % in maximum vertical velocity) andprecipitation intensity (up to 45 %), with the anthropogenic aerosoleffect more significant than the urban land effect. Urban land effectmodifies convective evolution: speed up the transition from the warm cloudto mixed-phase cloud, thus initiating surface rain earlier but slowing down the convective cell dissipation, all of which result from urban heating-induced stronger sea-breeze circulation. The anthropogenic aerosol effectbecomes evident after the cloud evolves into the mixed-phase cloud,accelerating the development of storm from the mixed-phase cloud to deepcloud by ∼ 40 min. Through aerosol–cloud interaction (ACI), aerosols boost convective intensity and precipitation mainly by activatingnumerous ultrafine particles at the mixed-phase and deep cloud stages. Thiswork shows the importance of considering both the urban land and anthropogenic aerosol effects for understanding urbanization effects on convective cloudsand precipitation. 

Abstract. Aerosol–cloud interactions (ACIs) are considered to be the most uncertaindriver of present-day radiative forcing due to human activities. Thenonlinearity of cloud-state changes to aerosol perturbations make itchallenging to attribute causality in observed relationships of aerosolradiative forcing. Using correlations to infer causality can be challengingwhen meteorological variability also drives both aerosol and cloud changesindependently. Natural and anthropogenic aerosol perturbations from well-defined sources provide “opportunistic experiments” (also known as natural experiments) to investigate ACI in cases where causality may be more confidently inferred. These perturbations cover a wide range of locations and spatiotemporal scales, including point sources such as volcanic eruptions or industrial sources, plumes from biomass burning or forest fires, and tracks from individual ships or shipping corridors. We review the different experimental conditions and conduct a synthesis of the available satellite datasets and field campaigns to place these opportunistic experiments on a common footing, facilitating new insights and a clearer understanding of key uncertainties in aerosol radiative forcing. Cloud albedo perturbations are strongly sensitive to background meteorological conditions. Strong liquid water path increases due to aerosol perturbations are largely ruled out by averaging across experiments. Opportunistic experiments have significantly improved process-level understanding of ACI, but it remains unclear how reliably the relationships found can be scaled to the global level, thus demonstrating a need for deeper investigation in order to improve assessments of aerosol radiative forcing and climate change. 

Abstract A multi-agency succession of field campaigns was conducted in southeastern Texas during July 2021 through October 2022 to study the complex interactions of aerosols, clouds and air pollution in the coastal urban environment. As part of the Tracking Aerosol Convection interactions Experiment (TRACER), the TRACER- Air Quality (TAQ) campaign the Experiment of Sea Breeze Convection, Aerosols, Precipitation and Environment (ESCAPE) and the Convective Cloud Urban Boundary Layer Experiment (CUBE), a combination of ground-based supersites and mobile laboratories, shipborne measurements and aircraft-based instrumentation were deployed. These diverse platforms collected high-resolution data to characterize the aerosol microphysics and chemistry, cloud and precipitation micro- and macro-physical properties, environmental thermodynamics and air quality-relevant constituents that are being used in follow-on analysis and modeling activities. We present the overall deployment setups, a summary of the campaign conditions and a sampling of early research results related to: (a) aerosol precursors in the urban environment, (b) influences of local meteorology on air pollution, (c) detailed observations of the sea breeze circulation, (d) retrieved supersaturation in convective updrafts, (e) characterizing the convective updraft lifecycle, (f) variability in lightning characteristics of convective storms and (g) urban influences on surface energy fluxes. The work concludes with discussion of future research activities highlighted by the TRACER model-intercomparison project to explore the representation of aerosol-convective interactions in high-resolution simulations.